Chemistry of Carbohydrates to Energy; Chemistry of Biomembranes; Chemistry of Ligands. Department of Chemistry, Princeton University, Princeton, NJ 08544 USA. 2Department of Biophysics, University of California, Los Angeles, CA 90095 USA. C.N.R. Author of the article. Affiliation: Department of Chemistry, University of Cambridge, Cambridge, CB3 2PP. Correspondence: Telephone:. E-mail: c.n.RJ
Abstract Sixty molecules of a carbonate salt (molecular formula: C 16 H 26), of the formula 1-(1,6-dibromopropylene-2,3-dihydro-2H-1,4-benzenediol-9,1,1,3-tetraazate -2,3-diethyl)-3,4-dimethylphenol, have been synthesized and characterized in this paper. Several are biodegradable, and a number have shown potential usefulness in the design of high-energy molecular fuel cells. In principle, a carbonate compound could be used to convert the electron-generating potential of an electrochemical cell to electrochemical current. Moreover, a carbonate compound could be used to convert the excess heat produced in an electrochemical cell to latent heat. In this context, the present study is aimed at testing the biodegradability and high yield of a carbonate compound. It was demonstrated that C 21 H 27 (1-(1,6-dibromopropylene-2,3-dihydro-2H-1,4-benzenediol-9,1,1,3-tetraazate -2,3-diethyl) was degraded to C 16 H 26 (1-(1,6-dibromopropyl)ethylcarbamate by microbial activity.
1. Introduction
Many biodegradable organic compounds were first generated by heat decomposition of organic products, including hydrogen peroxide, hydrogen peroxide (H 2 O 2) and the carboxylating alcohols ethylene glycol and cyclohexyl meth oxide [1]. A few of these compounds have been used as fuels, a typical example being ethylene glycol [1].
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THE JOURNAL OF BIOLOGICAL CHEMISTRY VOL. 281, NO. 15, pp. 9925 9934, April 14, 2006 2006 by The American Society for Biochemistry and Molecular Biology, Inc. Printed in the U.S.A. Cys-113 and Cys-422
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